Portable pneumatic systems for 2 degree-of-freedom (DOF) soft shoulder exosuits remain underexplored, and face fundamental trade-offs between torque output and dynamic response that are further compounded by the need for multiple actuators to support complex shoulder movement. This work addresses these constraints through a volume-optimized spindle-shaped angled actuator (SSAA) geometry: by reducing actuator volume by 35.7% (357mL vs. 555mL), the SSAA maintains 94.2% of output torque while achieving 35.2% faster dynamic response compared to uniform cylindrical designs. Building on the SSAA, we develop a curved abduction actuator (CAA) based on the SSAA geometry and a horizontal adduction actuator (HAA) based on the pouch motor principle, integrating both into a dual-DOF textile-based shoulder exosuit (390 g). The exosuit delivers multi-modal assistance spanning shoulder abduction, flexion, and horizontal adduction, depending on the actuation. User studies with 10 healthy participants reveal that the exosuit substantially reduces electromyographic (EMG) activity across both shoulder abduction and flexion tasks. For abduction with HAA only, the exosuit achieved up to 59% muscle activity reduction across seven muscles. For flexion, both the single-actuator configuration (HAA only) and the dual-actuator configuration (HAA,+,CAA) reduced EMG activity by up to 63.7% compared to no assistance. However, the incremental benefit of adding the CAA to existing HAA support was limited in healthy users during flexion, with statistically significant additional reductions observed only in pectoralis major. These experimental findings characterize actuator contributions in healthy users and provide design guidance for multi-DOF exosuit systems.

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