Prohibitive computational and environmental costs impede the scalable deployment of Large Language Models (LLMs). Traditional compression techniques (sparsity, quantization, low-rank approximations) are typically applied in isolation, and each hits an accuracy-efficiency wall. This thesis proposes the "Compression Trinity," a unified framework that applies the three pillars jointly: sparsity to reduce computation, quantization to minimize memory bandwidth, and low-rank approximations to recover accuracy. To accelerate pretraining, we apply the Trinity to the optimizer and model architecture. MKOR approximates curvature via block-diagonal sparsity and low-rank inversion, maintaining numerical stability for quantized states; it reduces curvature update complexity from $O(d^3)$ to $O(d^2)$ and accelerates convergence by up to 1.85x over KFAC. SLoPe accelerates training by up to 1.25x via a double-pruned backward pass for N:M sparsity, using low-rank "lazy" adapters in the final 1% of training to recover accuracy. For post-training compression, OPTIMA stabilizes static masks in a zero-training regime by formulating weight reconstruction as globally optimal column-wise quadratic programs, improving zero-shot accuracy by up to 3.97%. Given a fine-tuning budget, PATCH breaks the ceiling of static masks by learning a dynamic hybrid sparsity ratio between 0% and 50%, yielding up to 1.38x speedups. Finally, SLiM realizes the full Compression Trinity in one shot, using mathematically derived low-rank adapters to recover information lost to quantization and sparsity, improving accuracy by up to 5.66% over state-of-the-art methods and outperforming uncompressed dense models at equal parameter budgets by 0.6%. Together, these results show that jointly applying the Compression Trinity is essential for efficient, scalable, high-performance LLMs.

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