Estimating mutual information from text usually requires training a task-specific critic, which limits its use in low-data settings. We ask whether large language models can instead estimate pointwise mutual information zero-shot, using only prompts and elicited probabilities. We construct a benchmark from three publicly available human-annotated datasets with ground-truth PMI, and evaluate five information-theoretic prompting-based estimators. Our main method, PromptNCE, frames conditional probability estimation as a contrastive task and augments the candidate set with an explicit OTHER category. The OTHER category allows the model to assign probability mass outside the candidate set, avoiding the closed-set normalization of standard contrastive prompts. PromptNCE gives the best conditional probability estimates on all three datasets. For full PMI, we find that estimating label base rates is the primary bottleneck on two of the three datasets, with the best methods reaching Spearman correlation up to 0.78. We also present a case study in computer science education showing how these estimators can be used to score student knowledge summaries in a low-data setting. We release our code and prompts.

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