We develop a new framework for proving the undecidability of first-order theories of structures of the form $\langle \mathbb{N}; +, P \rangle$, $\langle \mathbb{N}; <, f \rangle$, and $\langle \mathbb{N}; +, f\rangle$, where $P \subseteq \mathbb{N}$ and $f \colon \mathbb{N} \to \mathbb{N}$. It is based on the recent proof of Hieronymi and Schulz that the first-order theory of $\langle \mathbb{N}; +, \{2^n \colon n \in \mathbb{N}\}, \{3^n \colon n \in \mathbb{N}\}\rangle$ is undecidable, and capable of transforming various randomness results about integer sequences into undecidability proofs. We apply our method to a large class of integer linear recurrence sequences, as well as various special functions, in particular showing that the first-order theories of $\langle \mathbb{N}; +, \{u_n \colon n \in \mathbb{N}\} \cap \mathbb{N}\rangle$, $\langle\mathbb{N}; <, n \mapsto \max\{0,u_n\}\rangle$, and $\langle \mathbb{N}; <, φ\rangle$ are undecidable, where $(u_n)_{n\in\mathbb{N}}$ is any integer LRS with exactly two non-repeated dominant roots satisfying a non-degeneracy assumption, and $φ$ is Euler's totient function.

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