Communication-centric ISAC is a promising paradigm for future 6G networks, in which data payload signals are expected to be reused for sensing to enhance time-frequency resource efficiency. For random payload signals, existing studies have mainly characterized the expected sidelobe level (ESL) of the periodic auto-correlation function (P-ACF). However, ESL only captures the average sidelobe behavior and does not control large spurious sidelobe peaks in individual payload realizations, which may deteriorate weak-target detection performance. This motivates the design of information-bearing signals whose random P-ACF satisfies stringent peak sidelobe level (PSL) constraints. In this paper, we formulate a mutual information maximization problem under PSL constraints and a power budget. For quasi-static frequency-flat channels, we show that a continuous auto-correlation function (ACF)-domain uniform construction provides an asymptotically optimal high-SNR design principle. Motivated by this principle, we propose auto-correlation function keying (ACFK), a finite-constellation modulation architecture that embeds data symbols directly onto the ACF-domain sidelobes. ACFK enables exact control of the nominal P-ACF, which coincides with the actual P-ACF when a spectral non-negativity constraint is met. When this is not the case, we quantify the non-negativity violation probability and bound the resulting peak sidelobe level ratio (PSLR) degradation. We further provide a reference ISAC transceiver design for ACFK over quasi-static multipath channels, together with high-SNR approximate BER analysis. Numerical results validate the theoretical analysis and show that, compared with a generalized probabilistic amplitude shaping (PAS) baseline, ACFK provides substantially stronger PSLR control and improved weak-target detection performance under comparable sensing and communication settings.

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