Electromagnetic (EM) methods, owing to their efficiency and non-invasive nature, have become one of the most widely used techniques in geological exploration. Nevertheless, data processing for these methods remains highly time-consuming and labor-intensive. With the remarkable success of deep learning, applying such techniques to EM methods has emerged as a promising research direction to overcome the limitations of conventional approaches. The effectiveness of deep learning methods depends heavily on the quality of datasets, which directly influences model performance and generalization ability. Existing application studies often construct datasets from random one-dimensional or structurally simple threedimensional (3D) models, which fail to represent the complexity of real geological environments. Furthermore, the absence of standardized, publicly available 3D geoelectric datasets continues to hinder progress in deep learning based EM exploration. To address these limitations, we present OpenEM, a large-scale, multi-structural 3D geoelectric dataset that encompasses a broad range of geologically plausible subsurface structures. OpenEM consists of nine categories of geoelectric models, spanning from simple configurations with anomalous bodies in half-space to more complex structures such as flat layers, folded layers, flat faults, curved faults and their corresponding variants with anomalous bodies. In addition, we provide a 3D model generator that enables fully controllable 3D model construction, allowing flexible and extensible augmentation of OpenEM. OpenEM provides a unified, comprehensive, and large-scale dataset for common EM exploration systems to accelerate the application of deep learning in electromagnetic methods. The complete dataset and 3D model generator is publicly available at https://doi.org/10.5281/zenodo.17141981.

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