Vision Transformers have achieved remarkable success in many fields, yet their deployment on edge devices remains challenging due to their substantial computational demands. Post-Training Quantization (PTQ) offers an attractive solution by compressing models using a small calibration set with minimal training overhead. However, most existing PTQ works adopt a static quantization paradigm that is uniformly applied to all instances. Given the substantial diversity of natural images, the activation distributions vary significantly across samples, making these methods inherently suboptimal. In this paper, we propose ScalePredictor, a dynamic quantization framework for accurate and efficient quantization scale learning of ViTs. We first reveal a hidden correlation between the distribution range of shallow-layer activations and the optimal scales of deeper layers. Based on this, we develop a scale learning mechanism that integrates an efficient range extraction approach to capture robust range statistics at the shallow stage, which are then fed into a Taylor-motivated polynomial scale projection module to generate all quantization scales simultaneously. With the efficiency of polynomial approximation, ScalePredictor introduces insignificant computational overhead while avoiding costly just-in-time calibration. Extensive experiments on ImageNet demonstrate that ScalePredictor consistently outperforms prior PTQ methods, achieving a more favorable accuracy-efficiency trade-off. Code and additional results are shown in the supplementary materials.

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