Large scale language model~(LLM) pretraining is increasingly bottlenecked by optimizer efficiency, driving optimizer design from vector-aware methods such as AdamW to matrix-aware methods. Matrix-aware optimizers such as Muon exploit matrix structure but treat layers independently, neglecting cross-layer correlations. Tensor-aware optimizers are therefore needed, yet existing ones rely on a matricization-based tensor algebra and remain restricted to shallow stacking and specific modules. In this paper, we propose \textbf{TUON}, a novel optimizer built on a transform-based tensor algebra derived from the Tensor-SVD (T-SVD). Unlike methods that polarize a globally unfolded matrix, TUON mixes layers via a unitary transform $\boldsymbol{Q}$ and then polarizes each transformed slice, and inverts the transform to recover the update. This mix-then-separate strategy captures cross-layer correlations while preserving per-layer diversity, avoiding the structural dimension imbalance and cross-layer misalignment of unfolding. Thus it successfully scales to more layers and diverse modules beyond QKV. Theoretically, we prove that TUON performs steepest descent under a $\boldsymbol{Q}$-transformed tensor spectral norm, and identify its update as the tensor polar factor of the T-SVD. We further establish transform non-redundancy, norm and smoothness comparisons with Muon and TEON, and a convergence guarantee. Empirically, TUON improves consistently over Muon and TEON on GPT-124M/350M and Qwen-0.6B/4B, with ablations confirming the transformation mechanism, cross-layer structure beyond two-layer stacking, adaptability beyond QKV, and robustness to the polarization method.

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