The collective behaviour of large language model (LLM) societies is not the sum of their individual outputs. It yields statistically distinct, sometimes-unpredictable phenomena, for which the tools we use to study single agents may not scale. Due to recent incidents involving autonomous agentic systems, however, understanding these systems is paramount. For that we introduce a framework for measuring self-organisation in LLM social systems and apply it to three such systems: a Schelling grid, a social network (Moltbook), and a Twitter-like misinformation simulation ('Rogue'). All three exhibit statistically significant self-organisation. Moreover, their relaxation dynamics vary with the environmental information available to the agents, with open-ended systems (Moltbook, Rogue) exhibiting sharp, phase-transition-like dynamics. Further results show that population-level pathologies can emerge even when the LLMs are safety-tuned or monitored, being primarily driven by the coordinated activity of a population subset. We also show when self-organisation does \textit{not} emerge under two additional scenarios (a commons dilemma, GovSim, and a LLM-as-a-judge deliberation scheme, ChatEval). We argue that measuring signatures of this kind offers a lightweight, agent-agnostic diagnostic layer for detecting coordinated collective behaviour in deployed multi-agent systems without relying on natural language or model versioning.

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