We prove a complexity dichotomy theorem for $\mathrm{Holant}^*$ problems over complex-valued symmetric constraint functions $\mathcal{F}$ on domain size $3$. We give a decidable tractability criterion and prove that if $\mathcal{F}$ satisfies the criterion, then $\mathrm{Holant}^*(\mathcal{F})$ is solvable in polynomial time, and otherwise it is #P-hard. This is the first Holant dichotomy for a set of complex-valued constraint functions on higher domains. We show that complex-valued constraint functions have a rich structure not observed in real-valued constraint functions. This structure is only revealed when we analyze them in a bipartite Holant setting with a non-standard bilinear form and provides the backbone to the proof of the dichotomy. We use group actions and the spin representation of $\mathrm{SL}(2, \mathbb{C})$ in $\mathrm{SO}(3, \mathbb{C})$ and the generalized orthogonal group to facilitate this analysis. We also introduce $\textit{frames}$ and $\textit{shells}$. Frames linearize the group action and provide a unified framework for proving #P-hardness when used in conjunction with shells. Furthermore, we characterize the lower dimensional constraint functions by $\textit{annihilators}$, which makes it possible to analyze $\textit{essentially Boolean domain}$ functions in domain size $3$.

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