Sparse computations are fundamental to scientific computing, graph analytics, and machine learning, yet their performance is highly sensitive to the diverse sparsity and patterns. This is because cache reuse, memory coalescing, and load balancing depend critically on the sparsity patterns. This work gives the first known exploration of the connections between sparse matrix computation and spectral analysis by treating sparse matrices as two-dimensional signals and analyzing their frequency-domain representations through Fast Fourier Transform. We show that spectral signatures uncover global structural characteristics that are not sufficiently captured by conventional spatial statistics and provide complementary information for understanding sparse computation performance. Experiments on incorporating spectral features into machine-learning-based SpMV format selection demonstrate the usefulness of such spectral analysis over a state-of-the-art spatial-only model. By uncovering the principled connections between spectral characteristics and sparse matrix computations, this work introduces a novel analytical perspective into sparse computation, and provides a new approach to enhancing the current sparse structure characterization and optimization. On pruned LLM decoding, adding spectral features improves kernel selection and yields 1.035--1.245$\times$ kernel speedups.

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