We develop new accelerated first-order algorithms in the Frank-Wolfe (FW) family for minimizing smooth convex functions over compact convex sets, with a focus on two prominent constraint classes: (1) polytopes and (2) matrix domains given by the spectrahedron and nuclear-norm balls. A key technical ingredient is a complementarity condition that captures solution sparsity---face dimension for polytopes and rank for matrices. We present two algorithms: (1) a purely linear optimization oracle (LOO) method for polytopes that has optimal worst-case first-order (FO) oracle complexity and, aside of a finite \emph{burn-in} phase and up to a logarithmic factor, has LOO complexity that scales with $r/\sqrtε$, where $ε$ is the target accuracy and $r$ is the solution sparsity (independently of the ambient dimension), and (2) a hybrid scheme that combines FW with a sparse projection oracle (e.g., low-rank SVDs for matrix domains with low-rank solutions), which also has optimal FO oracle complexity, and after a finite burn-in phase, only requires $O(1/\sqrtε)$ sparse projections and LOO calls (independently of both the ambient dimension and the sparsity level of optimal solutions). Our results close a gap on how to accelerate recent advancements in linearly-converging FW algorithms for strongly convex optimization, without paying the price of the dimension.

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