Omni-modal large language models (Omni-LLMs) extend LLMs to process heterogeneous modalities (e.g., vision, audio, and IMU signals) alongside language, enabling a broader range of multimodal tasks. Yet we find that these models often fail to express information from non-textual modalities even when they perceive it correctly. We term this disconnect knows-but-cannot-say. To investigate this phenomenon, we introduce Token-level Modality Alignment (TMA), which measures the alignment between individual modality representations and response representations. Our analysis shows that non-textual representations are less aligned with response tokens and receive less attention than textual representations, suggesting a potential explanation for uneven modality preferences. Motivated by these findings, we propose OmniCatalyst, a simple perceive $\rightarrow$ infer strategy that complements the original modality inputs with self-generated text, making non-textual knowledge more accessible. Across seven Omni-LLMs, OmniCatalyst consistently improves performance (+7.29%) and yields more balanced modality preferences, with further gains from diverse training strategies. Further analysis demonstrates that the knowledge extraction phases increase TMA, suggesting that improved alignment makes non-textual information more accessible during response generation. In summary, our findings uncover how Omni-LLMs can better express modality knowledge through language. Our code is available at https://github.com/naver-ai/OmniLLM.

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