We propose a causal machine learning framework to integrate dynamic tolling for mobility, equity, and climate objectives, resolving a long-standing policy trilemma. Using Double Machine Learning, we estimate zone-type-specific treatment effects, showing that commercial zones yield nearly twice the delay reduction of residential zones. Our adaptive quota mechanism expands residential coverage 34-fold while preserving 93% of total delay savings and sustaining high return on investment. The framework delivers climate co-benefits, reducing emissions by 743.5 metric tons of CO2 (valued at 141 USD) via congestion-sensitive pricing under moderate traffic conditions with sensitivity bounds from 557.6 to 929.3 tons. Crucially, we uncover a policy-invariant toll range where performance remains robust across demand scenarios, simplifying implementation. This study reveals critical, previously unidentified insights, such as a policy-invariant toll range, that can significantly simplify real-world implementation. Validated on synthetic data mirroring real-world networks, our methodological advances lay the foundation for future public deployment.

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